Use vROps for Automated Tagging

I am trying to find a way to use vROps 8.0.1 to identify machines that have a running process, and generate an alert if the process is running.

Is this possible?  Would it require Service Discovery, or Application Monitoring through the ARC Agent?

Essentially, what I would like to do, is create a custom group that contains the VMs running the certain process, so I can create an alert policy for them.